I greatly enjoyed uncharted vita. A bit on the easy side though.
Back to makin threads .....
THE BEST METHOD to run PSX games (and everything else for that matter) is via Retroarch - http://buildbot.libretro.com/nightly/
If you have any questions on how to set it up on Windows please feel free to ask, its very easy.
I'd really like the complete Uncharted set.